For me personally, I love using Titania. Especially in questing, she can be very broken on certain paths. As well as Hulkling too. All up to you though.
I'd say Iceman, he has a lot of immunities so it will help you if you are climbing story arc. Hulkling and Scorpion will also be solid investments, since they are not available at 7 star atm and being overall great champs. In the near future when you gets ascension dust, prioritize it for hulkling first, then scorpion and you should be good.
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