Most debuffs depend on crit rating (Iceman, Archangel, Killmonger, Wolverine, X-23, Black Panther,...). There are some champions that depend on crit damage (Crossbones, Corvus, Gamora).
It depends a bit on the champs you are using in your roster, but I think I went with Precision first. I had more champions at the time who benefited from being able to crit more often, as opposed to those who benefited from getting stronger crits.
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